Search for: All records

The emergent electronic, spin, and other quantum properties of 2D heterostructures of graphene and transition metal dichalcogenides are controlled by the underlying interlayer coupling and associated charge and energy transfer dynamics. However, these processes are sensitive to interlayer distance and crystallographic orientation, which are in turn affected by defects, grain boundaries, or other nanoscale heterogeneities. This obfuscates the distinction between interlayer charge and energy transfer. Here, nanoscale imaging in coherent four‐wave mixing (FWM) and incoherent two‐photon photoluminescence (2PPL) is combined with a tip distance‐dependent coupled rate equation model to resolve the underlying intra‐ and inter‐layer dynamics while avoiding the influence of structural heterogeneities in mono‐ to multi‐layer graphene/WSe₂ heterostructures. With selective insertion of hBN spacer layers, it is shown that energy, as opposed to charge transfer, dominates the interlayer‐coupled optical response. From the distinct nano‐FWM and ‐2PPL tip‐sample distance‐dependent modification of interlayer and intralayer relaxation by tip‐induced enhancement and quenching, an interlayer energy transfer time of  ps consistent with recent reports is derived. As a local probe technique, this approach highlights the ability to determine intrinsic sample properties even in the presence of large sample heterogeneity.

Stable high-power narrow-linewidth operation of the 2.05–2.1 µm GaSb-based diode lasers was achieved by utilizing the sixth-order surface-etched distributed Bragg reflector (DBR) mirrors. The DBR multimode devices with 100 µm wide ridge waveguides generated$\sim <\#comment/>850\mathrm{m}\mathrm{W}$in the continuous wave (CW) regime at 20°C. The device CW output power was limited by thermal rollover. The laser emission spectrum was defined by Bragg reflector reflectivity at all operating currents in a wide temperature range. The devices operated at DBR line with detuning from gain peak exceeding 10 meV.

A monochromatic wave that circulates in a nonlinear and dispersive optical cavity can become unstable and form a structured waveform. This phenomenon, known as modulation instability, was encountered in fiber lasers, optically pumped Kerr microresonators and, most recently, in monolithic ring quantum cascade lasers (QCLs). In ring QCLs, the instability led to generation of fundamental frequency combs—optical fields that repeat themselves once per cavity round trip. Here we show that the same instability may also result in self-starting harmonic frequency combs—waveforms that repeat themselves multiple times per round trip, akin to perfect soliton crystals in ring Kerr microresonators. We can tailor the intermode spacing of harmonic frequency combs by placing two minute defects with a well-defined separation between them along the ring waveguide. On-demand excitation of frequency comb states with few powerful modes spaced by hundreds of gigahertz may find their use in future sub-terahertz generators.